2024
DOI: 10.21203/rs.3.rs-3991307/v1
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Transient Pulsed Discharge Preparation of Graphene Aerogel Supported Asymmetric Cu Cluster Catalysts Promote CO2 Reduction to Ethanol

Wenxing Chen,
Kaiyuan Liu,
Hao Shen
et al.

Abstract: Precisely designing asymmetrical structure is an efficient strategy to optimize the performance of metallic catalysts for electrochemical carbon dioxide reduction reactions. Herein, a transient high-density current induced by pulsed discharge is used to rapidly construct graphene aerogel (GAs) supported asymmetric Cu cluster catalysts. Cu atoms decomposed by CuCl2 are converged on graphene surfaces in GAs together with oxygen originating from the intense current and instantaneous high temperature. The atomic a… Show more

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