Transition metal catalysed cascade C–C and C–O bond forming events of alkynes

Barik, Padmanava; Behera, Subhra Sriharsa; Nayak, Laxmi Kanta; Nanda, Laxmi Narayan; Nanda, Santosh Kumar; Patri, Padmanava

doi:10.1039/d3ob02044d

Org. Biomol. Chem.

2024

DOI: 10.1039/d3ob02044d

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Transition metal catalysed cascade C–C and C–O bond forming events of alkynes

Padmanava Barik,

Subhra Sriharsa Behera,

Laxmi Kanta Nayak

et al.

Abstract: The past few decades have seen the emergence of domino reactions as a powerful tool for the multi-functionalization of alkynes for the rapid and smooth construction of complex molecular architectures....

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2024

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Cited by 3 publications

References 133 publications

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Manganese-Catalyzed Cycloalkene Ring Expansion Synthesis of Azaheterocycles

Wang,

Xu,

Han

et al. 2024

Org. Lett.

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Herein, a Mn catalytic protocol has been developed for the cycloalkene ring expansion synthesis of azaheterocycles, allowing broad-substrate-scope access to pyridine and isoquinoline derivatives. The initial monoaddition of an azidyl radical to alkene and further as-generated C-radical addition to O 2 , followed by intramolecular rearrangement and aromatization, showcase a distinct Mn-catalyzed radical reactivity mode. The reaction features a short reaction time and a broad substrate scope, with applications demonstrated in complex structure elaboration and gram-scale vismodegib synthesis.

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Manganese-Catalyzed Cycloalkene Ring Expansion Synthesis of Azaheterocycles

Wang,

Xu,

Han

et al. 2024

Org. Lett.

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Silver-Catalyzed Markovnikov Addition Hydrofunctionalization of Terminal Alkynes: Synthesis of N-Enoxyimides and Oximes

Noor,

Zhang,

Jia

et al. 2024

Org. Lett.

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Efficient and regioselective synthesis of ortho-diiodinated homobenzylic alcohol derivatives: in silico evaluation as potential anticancer IDO/TDO inhibitors

Al-Zoubi,

Al-Jammal,

Shkoor

et al. 2024

Org. Biomol. Chem.

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Transition metal catalysed cascade C–C and C–O bond forming events of alkynes

Abstract: The past few decades have seen the emergence of domino reactions as a powerful tool for the multi-functionalization of alkynes for the rapid and smooth construction of complex molecular architectures....

Cited by 3 publications

References 133 publications

Manganese-Catalyzed Cycloalkene Ring Expansion Synthesis of Azaheterocycles

Manganese-Catalyzed Cycloalkene Ring Expansion Synthesis of Azaheterocycles

Silver-Catalyzed Markovnikov Addition Hydrofunctionalization of Terminal Alkynes: Synthesis of N-Enoxyimides and Oximes

Efficient and regioselective synthesis of ortho-diiodinated homobenzylic alcohol derivatives: in silico evaluation as potential anticancer IDO/TDO inhibitors

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