can efficiently couple light into nanostructures and confine light below diffraction limit. [8,9] With these properties, plasmonics have found important applications in various fields such as plasmonic sensing, [10][11][12][13] plasmon-enhanced spectroscopies, [14][15][16] plasmonic nanolasing, [17][18][19] and perfect light absorption. [20,21] The optical performances of plasmonic nanostructures are highly dependent on the resonance modes that they support. Generally, there are two fundamental surface plasmonic modes: localized surface plasmon resonance (LSPR) and propagating surface plasmon polaritons (SPP). [22,23] LSPR can be observed on metal nanoparticles. [22,24,25] However, the strong radiative damping of metal nanoparticles results in broad resonant spectra, severely limiting the applications of metal nanoparticles in fields such as plasmonic sensing and nanolasing. [26,27] SPP is usually generated at the interface between metal and dielectric with the assistance of a high refractive index prism or by constructing a grating structure. [23,28,29] The near-field decay length of SPP mode is 40-50 times larger than that of LSPR mode. [23] Therefore, SPP structures usually provide higher bulk sensitivity when used for plasmonic sensing. [23] However, it is difficult to achieve a flexible tuning of SPP mode only by above configurations. In addition, single resonance mode also greatly limits the applications of the devices.According to the plasmon hybridization theory, coupling of different resonance modes can endow plasmonic nanostructures with richer optical properties and thereby improve their performance and broaden their application fields. [30][31][32] Metallic plasmonic arrays have been demonstrated to be a powerful platform for the simultaneous excitation of the above two basic types of plasmonic modes. [33,34] In addition, they can also support many other types of resonance modes such as Fabry-Pérot (F-P) cavity mode, surface lattice resonance (SLR), and plasmonic Fano resonance due to the flexibility in structure design. [32,[35][36][37][38] These modes together give the nanostructured plasmonic arrays with attractive performance unattainable by using individual LSPR or SPP mode. Benefited from the abundant optical properties, nanostructured metallic plasmonic arrays can be utilized in a fashion of "device-by-design." For example, for plasmonic sensing, a plasmonic array with a narrow spectrum can be fabricated for an excellent sensing performance; [23,26] while for surface-enhanced Raman spectroscopy (SERS) detection, a plasmonic array with a relatively broad spectrum is needed to achieve local field enhancement and radiative enhancement simultaneously. [39,40] Therefore, the investigation The vast development of nanofabrication has spurred recent progress for the manipulation of light down to a region much smaller than the wavelength. Metallic plasmonic array structures are demonstrated to be the most powerful platform to realize controllable light-matter interactions and have found wide application...