We report measurements on a silicon nanowire quantum dot with a clarity that allows for a complete understanding of the spin states of the first four holes. First, we show control of the hole number down to one. Detailed measurements at perpendicular magnetic fields reveal the Zeeman splitting of a single hole in silicon. We are able to determine the ground-state spin configuration for one to four holes occupying the quantum dot and find a spin filling with alternating spin-down and spin-up holes, which is confirmed by magnetospectroscopy up to 9T. Additionally, a so far inexplicable feature in single-charge quantum dots in many materials systems is analyzed in detail. We observe excitations of the zero-hole ground-state energy of the quantum dot, which cannot correspond to electronic or Zeeman states. We show that the most likely explanation is acoustic phonon emission to a cavity between the two contacts to the nanowire. 1 arXiv:0811.2914v1 [cond-mat.mes-hall]
Nov 2008Long spin lifetimes are crucial for applications such as spintronics [1] and even more so for quantum computation with single spins. The proposal to use single spins as quantum bits [2,3] exploits an optimal combination of the spin and charge degree of freedom [4]. The potential of this spin qubit is underlined by the recent demonstration of coherent control of one [5] and two [6] spin states in quantum dots in GaAs/AlGaAs heterostructures. Most experiments have focused on quantum dots formed in III-V semiconductors; however, electron spin coherence in those materials is limited by hyperfine interactions with nuclear spins and spin-orbit coupling. Group IV materials are believed to have long spin lifetimes because of weak spin-orbit interactions and the predominance of spinzero nuclei. This prospect has stimulated significant experimental effort to isolate single charges in carbon nanotubes [7,8], Si FinFETs [9] and Si nanowires [10]. The recent observation of spin blockade in Si/SiGe heterostructures is argued to confirm the predicted long-lived spin states [11]. Here we identify the spin states of single charges in silicon quantum dots by means of low-temperature electronic transport experiments, for the first time to the level of individual spin states.We have measured 30 Si nanowire quantum dots with pronounced excited states. In the measurements presented here, both a backgate and a side gate allow control of the number of charges down to a single hole in the dot. We observe the Zeeman energy of the first two holes at magnetic fields ranging from 0 to 9 T, from which we deduce a g-factor close to the Si bulk value. Magnetospectroscopy of the first four holes allows determination of the successive spins that are added to an empty dot and reveals a spin filling with alternating spin-down and spin-up holes. The isolation and identification of a single spin in silicon demonstrated here constitutes an important step towards spintronic applications in a material with a long spin coherence time. Additionally, we have identified many ex...