Direct observation of domain wall (DW) nucleation and propagation in focused electron beam induced deposited Co nanowires as a function of their dimensions was carried out by Lorentz microscopy (LTEM) upon in situ application of magnetic field. Optimal dimensions favoring the unambiguous DW nucleation/propagation required for applications were found in 500-nm-wide and 13-nm-thick Co nanowires, with a maximum nucleation field and the largest gap between nucleation and propagation fields. The internal DW structures were resolved using the transport-ofintensity equation formalism in LTEM images and showed that the optimal nanowire dimensions correspond to the crossover between the nucleation of transverse and vortex walls. In the last decade, several pioneering works envisaged different strategies to design magnetic information storage, logic devices or sensors based on magnetic domain walls (DW) as functional entities to store, transfer, and process information in ferromagnetic media. [1][2][3][4][5] These innovative ideas and promising applications have motivated extensive developments of ferromagnetic nanostructures in which DW can be "easily" created and driven either by external magnetic fields and/or spin-polarized currents. 6-12 DW in magnetic nanostructures have therefore become a major topic for the research community in the field of Nanomagnetism. The specific DW configuration is the result of the balance between the magnetostatic energy, the magnetocrystalline anisotropy, and the exchange coupling. Therefore, along with the intrinsic properties of the magnetic material, it also depends on the geometry and the dimensions of the nanostructures. 13 In magnetic nanowires (NWs), the possible DW configurations are either symmetric or asymmetric transverse walls (TWs) or vortex walls (VWs) and they move differently under the application of an external magnetic field or current. 14 Therefore, a careful analysis of the DW structure of devices as a function of dimensions, geometries, shape of constrictions, etc. is requested to determine the type of magnetic configurations appearing in a given nanostructure and the possibility of tuning and manipulating them upon the application of external magnetic fields or electric currents. 6,8,[10][11][12] Permalloy (Py) nanostructures have been extensively studied because of their low magnetocrystalline anisotropy, thus allowing the control of its magnetic properties simply adjusting its shape anisotropy. Therefore, many Py nanostructures of various shapes and sizes have been synthetized using electron beam or UV lithography processes. [1][2][3][4][5][6][7][8][9][10][11][12]15,16 The use of ferromagnetic materials alternative to Py and the development of advanced nanofabrication methods allowing creating magnetic nanostructures of dimensions less than 100 nm are however needed to explore their functionalities and possible applications. In the last years, focused electron beam induced deposition (FEBID) technique has demonstrated a capacity to produce high quality nanostructu...