growth with severe electrolyte consumption in most liquid organic electrolytes, especially in carbonate-based ones. [4][5][6][7] To realize viable application of Li metal anodes, continuous effort has been made for years to understand the mechanism of Li deposition and tackle the formation of dendrites. [8][9][10][11] To this end, much work has been devoted in designing Li hosts and substrates, [12][13][14][15] using electrolyte additives [16][17][18][19][20] or solid electrolytes, [21][22][23] and introducing protection films. [24][25][26][27][28][29] For examples, Guo et al. reported that 3D Cu with a large number of charge centers and nucleation sites facilitate the formation of relatively even Li surface. [12] Zhang and co-workers demonstrated a self-healing electrostatic shield mechanism for dendrite-free lithium deposition by controlling Li-ion diffusion on the electrode surface. [20] In recent years, the effect of charging methods on suppressing dendrite growth during Li deposition has attracted increasing attention. [30][31][32] He et al. studied the effectiveness of pulse current charging on dendrite suppression by choosing proper on/ off times of the pulses. [30] Whittingham and co-workers also showed that pulse current charging improves lithium cycling efficiency under diffusion-controlled conditions. [31] Miller et al. employed a coarse-grained simulation model to prove that shorter pulse durations can lead to lower tendency of dendrite formation. [32] This is further confirmed by Hoffmann et al. who demonstrated that 1 ms pulse charging can inhibit the dendrite propagation more effectively than 20 ms pulse or constant current charging. [33] A more recent work by Maraschky and Akolkar indicated that pulsed current may mitigate the concentration depletion of Li ions within the solid electrolyte interphase (SEI), because the diffusion time constant of Li ions has a value of 1 ms for a 10 nm thick SEI and thereby the concentration gradient of Li ions formed across the SEI during charging can be nullified within 1 ms of rest period. [34] The above simulation and experimental studies suggest that interval charging could improve homogeneous nucleation of Li by controlling the diffusion process, therefore high-frequency pulse charging is beneficial for suppressing the growth of Li dendrites.Recently, rotary triboelectric nanogenerators (R-TENGs) originating from contact electrification have been developed and successfully demonstrated as mechanical energy harvesters. [35][36][37] A unique character of R-TENGs is that their voltage and current outputs are high-frequency sinusoidal waveforms. Despite that the effect of sinusoidal ripple current