2020
DOI: 10.1016/j.jechem.2019.06.005
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Trithiocyanuric acid derived g–C3N4 for anchoring the polysulfide in Li–S batteries application

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Cited by 68 publications
(32 citation statements)
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“…[19] Besides, in contrast to graphene and carbon nanotubes, the presence of Lewis-base pyridine nitrogen in C 3 N 4 can effectively interact with the strong Lewis-acid of terminal Li atoms in LiPS, thus contributing to prolonging the lifespan of LSBs. [20][21][22] In terms of geometric structure, graphite C 3 N 4 nanosheets (s-CN) prepared by the traditional liquid-phase exfoliation method usually suffer from low SSA due to re-aggregation by van der Waals forces. [23] On the other hand, template methods to produce high-SSA C 3 N 4 are cumbersome and wasteful, inappropriate for a technology with a huge potential market and thus potentially requiring enormous amounts of materials.…”
Section: Introductionmentioning
confidence: 99%
“…[19] Besides, in contrast to graphene and carbon nanotubes, the presence of Lewis-base pyridine nitrogen in C 3 N 4 can effectively interact with the strong Lewis-acid of terminal Li atoms in LiPS, thus contributing to prolonging the lifespan of LSBs. [20][21][22] In terms of geometric structure, graphite C 3 N 4 nanosheets (s-CN) prepared by the traditional liquid-phase exfoliation method usually suffer from low SSA due to re-aggregation by van der Waals forces. [23] On the other hand, template methods to produce high-SSA C 3 N 4 are cumbersome and wasteful, inappropriate for a technology with a huge potential market and thus potentially requiring enormous amounts of materials.…”
Section: Introductionmentioning
confidence: 99%
“…The strong flexibility of the 2D monolayer material enhanced the possibility of molecular adhesion, improved electron mobility and leaded to a smaller interface impedance with sulfur electrode. In addition to graphene and CNT, other 2D materials (COFs, [83] MOFs [64,78,81,114] (Figure 5i), MXene, [57,115] C 3 N 4 [116] (Figure 5g), etc.) are utilized to ornament the cathodes.…”
Section: Other Namomaterialsmentioning
confidence: 99%
“…Apart from that, g-C 3 N 4 also holds advantages of light weight and high porosity over the popularly-studied inorganic LiPS adsorbents such as metal oxides, carbides, sulfides, and nitrides. In view of these benefits, several attempts of cathode construction or separator modification by g-C 3 N 4 have been explored with considerable improvements [22][23][24][25][26][27]. However, the generally planar or particulate g-C 3 N 4 suffers from either insufficient physical sulfur accommodation or limited active site exposure.…”
Section: Introductionmentioning
confidence: 99%