“…Many more two‐dimensional (2D) materials are continuing emerging with a rainbow of intriguing physical properties including excellent photoluminescence (PL) emission 1 (e.g., MoS 2 and MoSe 2 ), superconductivity 2,3 (e.g., NbS 2 and TaS 2 ), magnetism 4–6 (e.g., CrI 3 and NiPS 3 ), and ferroelectricity 7,8 (e.g., CuIn 2 PS 6 ). Moreover, stacking these 2D materials in different configurations—vertically or horizontally—leads to the formation of various homostructures and heterostructures with tunable electronic, optical, and magnetic properties 9–13 …”