“…If melt growth is eschewed because of these assorted shortcomings, the next most common growth techniques dissolve the feedstock under conditions well below the melting point and then crystallize out the feedstock from the solution. Chemical vapor deposition (CVD) or chemical transport (UO 2 , − U x Th 1– x O 2 , and U 1– x Pu x O 2 ), flux (CeO 2 , − ThO 2 , ,,− ,− UO 2 , ,, U x Th 1– x O 2 , and PuO 2 ,− ), and hydrothermal or solvothermal synthesis (CeO 2 , ThO 2 , ,,,− U 1– x Th x O 2 , − UO 2 , − ,− and PuO 2 ) fall into this category and have been employed for the entire AO 2 family. High-quality, well-faceted single crystals of ThO 2 and UO 2 produced using the hydrothermal method are shown in Figure .…”