2024
DOI: 10.1002/cssc.202401606
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Two‐Dimensional π‐d Conjugated Conductive Metal‐Organic Framework with Triple Active Centers as High‐Performance Cathodes for Flexible Zinc Batteries

Hong Ding,
Ping Liu,
Chengyu Liu
et al.

Abstract: Conductive metal‐organic frameworks (C‐MOFs) have received extensive interest in high‐performance zinc‐ion batteries (ZIBs) owing to multi‐redox sites and high electrical conductivity. Here, we present a π−d C‐MOF by coordinating 2,3,5,6‐tetraaminobenzoquinone (TABQ) ligands with Cu2+ ions (2D Cu‐TABQ) acting as cathodes for ZIBs. Benefiting from a triple active center (Cu2+, C=O, and C=N), 2D Cu‐TABQ shows an ultra‐high reversible capacity of 297.7 mAh g‐1at 0.2 A g‐1. Meanwhile, 2D Cu‐TABQ also has superior … Show more

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