Due to the exceptional multiphase
mixing and mass transfer performance,
gas–liquid vortex units (GLVUs) have great potential for solvent-based
applications such as CO2 capture. The high gas flow rates
needed to provide the energy input for creating the centrifugal field
negatively influence the contact between phases and the efficiency
of the GLVU. To address this issue, computational fluid dynamics (CFD)
simulations are used to optimize the design of the GLVU geometry and
its operating conditions. The gas–liquid flow characteristics,
contact time, and total energy consumption in different GLVU geometries
are analyzed. The effects of geometrical changes including reactor
shape, reactor volume, and gas–liquid inlet configuration are
investigated. In the optimized GLVU designs, the gas–liquid
contact time is increased by more than a factor of 3, while the energy
consumption is reduced by 85%, compared to the base case. Structural
optimization of a GLVU is an effective route to improve the gas–liquid
contact time. The use of CFD significantly accelerates the optimization
of the design of a GLVU geometry for subsequent manufacturing.