Considering the inadaptability of traditional anodic bonding to polymer materials, the flexible anodic bonding process is developed. The bonding characteristics of the dynamic intelligent electric fields with the low-temperature plasma surface treatment to polymer and ultrasonic-assisted preconnection before bonding are very suitable for the anodic bonding of polymer elastomer to aluminum (Al) sheet. A series of composite polyurethane elastomer cathode materials (CPECs) with good bonding properties are prepared and characterized. The highest ionic conductivity of CPECs can reach to 2.7 Â 10 À3 S/cm (CPEC2) at 75 C. After bonded, it is determined that a uniform and dense intermediate bonding layer showed by SEM is formed between CPECs and Al. In addition, different elements including C, O, F, S, and Al are clearly iden-