an emerging material, liquid metal when used in combination with polydimethylsiloxane (PDMS) finds applications in soft/ flexible and wearable electronics. [2] Due to its flexibility and deformability, liquid metal encapsulated in PDMS has recently shown self-healing characteristics after damage on the device. [7][8][9] Gallium-based liquid metal has been explored in various applications ranging from electrocardiogram, [10] microcooling, [11] thermometers, [12] flexible electrodes, [13,14] flexible interconnection, [15] strain sensors, [16] pressure sensors, [17] inkjet printing, [18] energy harvesting, [19,20] and magneto-hydrodynamic pumps. [21] Metasurface-based frequency selective surface (FSS) exists in 1D or 2D as periodic arrays of sub-wavelength metallic elements on dielectric surfaces. [22,23] Based on material, physical construction, [24] and geometry, [25] the FSSs are classified into high-pass, low-pass, band-pass, and bandstop filter. [25,26] The performance and behavior of the FSS is dependent on the geometry, periodicity, array size, and choice of materials (conductivity and permittivity). [24] The FSSs have been extensively studied [27] since 1960s, however its fundamental origin can go back to Marconi and Franklin's patent of reflectors in 1919. [28] The ability to tailor FSSs to curtail certain frequency band makes it a vital component in communication applications including radar, [23,29,30] microwave absorber, [29] satellite, [23,31] electromagnetic interference shielding, [32] dichroic sub reflectors, [33] reflect array lenses, [34] lens antenna, [35] polarizers, [36] stealth blankets, [37] and wireless networks. [23,38] Traditional metasurfaces have been realized on rigid substrates using materials such as glass, [23] quartz, [39] polytetrafluoroethylene (PTFE) reinforced with glass, [40] commercially available FR-4-based printed circuit boards, [41][42][43] Rogers 5880 PTFE composites supported with glass microfibers. [44] The varactor diodes like BB 837 or BB 857-02 V, [41,45] liquid crystal, [40,46] and silver paint were either soldered, [41] filled/deposited, [40,46] or painted into these mechanically rigid substrates. [23,47] Recently, liquid metal injection in all connected microfluidic channels in PDMS has been used to realize physically flexible metasurfaces with or without incorporation of soldered chip resistors. [48,49] While the metasurface is flexible, serial injection/withdrawal of liquid metal in all connected microfluidic channels may limit its application (e.g., metasurface that needs unconnected patterns). Injection filling is also known for leaving airgaps and may cause device delamination. [50] A flexible self-healing metasurface using gallium-based liquid metal encapsulated in polydimethylsiloxane (PDMS) operating in the X-band (8-12 GHz) is reported. A band-stop metasurface with center frequency at 9.82 GHz is designed using floating patches surrounding the respective end cap of a Jerusalem cross. A large-scale (up to 10 × 10 array) metasurface is patterned in PDMS and ...