2015
DOI: 10.1038/ncomms7150
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Ultrasensitive and label-free molecular-level detection enabled by light phase control in magnetoplasmonic nanoantennas

Abstract: Systems allowing label-free molecular detection are expected to have enormous impact on biochemical sciences. Research focuses on materials and technologies based on exploiting localized surface plasmon resonances in metallic nanostructures. The reason for this focused attention is their suitability for single molecule sensing, arising from intrinsically nanoscopic sensing volume, and the high sensitivity to the local environment. Here we propose an alternative route, which enables radically improved sensitivi… Show more

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Cited by 186 publications
(198 citation statements)
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“…A remarkable exception is their application to label-free molecular detection. In this case, despite the smallness of MO activity and large losses, MP crystals and nanoantennas were found to enable a radically improved sensitivity, clearly outperforming conventional plasmon based sensors [104]. The key challenge is to increase the strength of SO coupling without increasing the plasmon damping, due to dissipative losses.…”
Section: Magneto-plasmonicsmentioning
confidence: 99%
“…A remarkable exception is their application to label-free molecular detection. In this case, despite the smallness of MO activity and large losses, MP crystals and nanoantennas were found to enable a radically improved sensitivity, clearly outperforming conventional plasmon based sensors [104]. The key challenge is to increase the strength of SO coupling without increasing the plasmon damping, due to dissipative losses.…”
Section: Magneto-plasmonicsmentioning
confidence: 99%
“…the rotation and ellipticity of light polarization upon transmission or reflection. Phase-sensitive detection of the magneto-optical signal provides a sensitive method for biosensing at the molecular level, as recently demonstrated for cylindrical Ni nanoantennas [14].…”
Section: Introductionmentioning
confidence: 99%
“…Hence, it is difficult to achieve ferromagnetic and plasmonic behaviors in the same material. Only recently, nanostructures of Ni [14][15][16][17][18][19][20] Ni/Co [21] and permalloy antidots [22] have been reported to exhibit surface plasmons in combination with their well-known ferromagnetic character at room temperature. However, the intensity of the plasmonic resonance in these type of materials is fairly weaker than for noble metals as Au or Ag where the electromagnetic field can be increased locally up to 80 times upon excitation of surface plasmons [23].…”
Section: Introductionmentioning
confidence: 99%