2014
DOI: 10.1364/ol.39.000383
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Ultrashort optical pulse characterization using WS_2 monolayers

Abstract: We demonstrate the application of two-dimensional materials for ultrashort optical pulse characterization. Monolayer transition metal dichalcogenides, such as tungsten disulfide (WS₂), possess extraordinarily large second-order nonlinear susceptibility, and due to their atomic thickness, have relaxed phase-matching requirements and, hence, an inherently wide bandwidth. Synthesized monolayer WS₂ triangular islands were used to characterize ultrashort optical pulses at the focal point of an objective lens throug… Show more

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Cited by 34 publications
(22 citation statements)
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“…TMDs include some metals, various semiconductors, as well as superconductors. Over years of development, studies of TMDs have mainly concentrated on MoS 2 , MoSe 2 , WS 2 , and WSe 2 [7][8][9]. They have a changed characteristic (such as electronic structure, band gap) with their different layer thickness, owing to interlayer interactions and the variations of screening.…”
Section: Introductionmentioning
confidence: 99%
“…TMDs include some metals, various semiconductors, as well as superconductors. Over years of development, studies of TMDs have mainly concentrated on MoS 2 , MoSe 2 , WS 2 , and WSe 2 [7][8][9]. They have a changed characteristic (such as electronic structure, band gap) with their different layer thickness, owing to interlayer interactions and the variations of screening.…”
Section: Introductionmentioning
confidence: 99%
“…Very recently, monolayer WS 2 showed an extraordinarily large second-order nonlinear susceptibility [17]. And WS 2 monolayers have been used for ultra-short optical pulse characterization via second harmonic generation [18]. While MoS 2 has received increasing attention for ultra-short pulse generation, little attention has been paid to WS 2 nano-sheets and WS 2 -based Q-switched fiber laser has not been reported, to the best of author's knowledge.…”
Section: Introductionmentioning
confidence: 99%
“…WS 2 also exhibits strong spin-orbit coupling and band splitting due to spin enabling spintronics/valleytronics, which was first demonstrated in MoS 2 22 23 24 . WS 2 also has high nonlinear susceptibility, suggesting its use for nonlinear optical devices 25 26 . However, most device research to date has been largely based on mechanically exfoliated layers which does not allow high throughput manufacturing.…”
mentioning
confidence: 99%