Lap shear joints comprised of aluminum-aluminum, aluminum-glass fiber-reinforced polymer (GFRP), aluminum-carbon fiber-reinforced polymer (CFRP), CFRP-CFRP, CFRP-GFRP and GFRP-GFRP, were exposed to 95% relative humidity (RH) at 50 • C, 70 • C and 90 • C, to salt fog and to a 90 • C/95%RH freeze cycle. Electrochemical impedance spectroscopy (EIS) spectra were taken across the whole bonded assembly using an EIS corrosion sensor. Periodically, some specimens were pulled to obtain bond strength as a function of exposure. As expected, the higher the temperature, the faster the bond degradation. The low-frequency impedance correlated with bond strength of the humidity-exposed specimens and showed the same Arrhenius dependence, suggesting that moisture absorption by the adhesive was the limiting factor in bond performance and that EIS has the potential to nondestructively track bond health and warn of deterioration.