We report neutron diffraction measurement results for an Ising antiferromagnet CoNb 2 O 6 under uniaxial pressure along the geometrically frustrated isosceles-triangular-lattice direction. We find that an onset incommensurate wave number at the Néel temperature increases with pressure from 0.378 to 0.411 at 400 MPa. The observations suggest that the anisotropic deformation of the lattice by the uniaxial pressure significantly modifies the spin frustration, leading to an increase in the nearest-neighbor to next-nearest-neighbor interaction ratio from 1.33 to 1.81.Geometrically frustrated triangular-lattice antiferromagnets (TLAs) have been attracting considerable interest because of their diverse phase transitions and critical phenomena [1,2] as well as the recent discovery of multiferroics properties in some TLAs [3][4][5]. For an ideal two-dimensional (2D) triangular lattice with a nearest-neighbor antiferromagnetic interaction, no long-range magnetic order occurs in the case of Ising spins, even at T = 0 K, owing to macroscopic degeneracy of the ground state, whereas a 120 • structure is expected to be stabilized at T = 0 K for Heisenberg or XY-type spins. On the other hand, real TLAs usually exhibit magnetic orders at nonzero temperature, irrespective of spin type, and the phase transition is three dimensional in nature due to the stacking structure of the frustrated triangular lattice. Moreover, there exist other microscopic interactions, such as further-neighbor and dipole-dipole interactions, which reduce the degeneracy of the ground state. Nevertheless, the triangular geometrical frustration does dominate the magnetic order and diverse magnetic features have been experimentally determined in a variety of TLAs [2].A partial releasing of the triangular geometrical frustration due to an orthorhombic distortion also has pronounced effects on magnetic ordering. This distortion splits J on a triangular lattice into two inequivalent antiferromagnetic interactions, J 1 and J 2 , on an isosceles-triangular lattice, as shown in Fig. 1(b). Theoretical investigation of a 2D Ising isosceles-triangular lattice revealed interesting magnetic features, which depend on the interaction ratio, γ = J 1 /J 2 [6-8]. Simple long-range antiferromagnetism is achieved for γ < 1.0 of the triangular lattice, whereas for γ > 1.0 the system only shows a longrange order at T = 0 K, with decoupled chains along the J 1 direction. Above this temperature, magnetic correlations between the chains and an incommensurate magnetic order are seen. The investigation of magnets with geometrically * koba@iwate-u.ac.jp frustrated isosceles-triangular lattices is of great importance, because such a system does not simply belong to the intermediate case between the geometrically frustrated TLA and unfrustrated magnet, but it also has the potential to exhibit unusual magnetic features absent in both magnets.In this Rapid Communication, we report the results of neutron diffraction measurements on an isosceles-triangularlattice Ising antiferromagnet, CoNb ...