“…The study of interactions between flying free electrons and quantized systems, such as electromagnetic fields or bound electrons, has led to the emerging field of free-electron quantum optics . − Free-electron quantum optics provides a promising platform for the generation of nonclassical light, ,,,− quantum information processing, − and quantum sensing. ,,,,− Specifically, measurement of free electrons’ energy can be used for the heralded generation of quantum light, such as Fock states, ,,,,− squeezed states and even cat and GKP states . More recently, it was predicted that free electrons could serve as ancillary qubits for quantum computation , and provide a platform for nonlinear electron dynamics , and deterministic single-photon nonlinearities ,, emerging from quantum recoil. , Owing to the nature of free-electron emitters, the anticipated single photon nonlinearity can span a vast spectral range , and operate on femtosecond-temporal and subwavelength-spatial resolution, − allowing new paradigms in quantum optical technologies.…”