2024
DOI: 10.1002/adfm.202418021
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Unraveling the Synergy of Au and Polar MgO(111) Surface in Photothermal Catalytic Oxidative Coupling of Methane

Tianyang Shen,
Siyu Hu,
Xiaoliang Sun
et al.

Abstract: Direct and selective catalytic oxidative coupling of methane (OCM) into high‐carbon products is a great challenge in C1 chemistry. Herein, the successful fabrication of a series of Au clusters loaded on different MgO facets of (111), (110), and (100) is reported. This work demonstrates the Au‐loaded MgO(111) (denoted as Au/MgO(111)) shows the highest C2H6 yield of 12733.4 µmol g−1 h−1 and selectivity of 90.4%, which is 2.46 times higher than that of Au/MgO(110) (5171.4 µmol g−1 h−1) and 25.14 times higher than… Show more

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