Unraveling the ultrafast dynamics of thermal-energy chemical reactions

Robinson, Matthew S.; Küpper, Jochen

doi:10.1039/d3cp03954d

Phys. Chem. Chem. Phys.

2024

DOI: 10.1039/d3cp03954d

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Unraveling the ultrafast dynamics of thermal-energy chemical reactions

Matthew S. Robinson,

Jochen Küpper

Abstract: In this perspective, we discuss how one can initiate, image, and disentangle the ultrafast elementary steps of thermal-energy chemical dynamics, building upon advances in technology and scientific insight. We propose...

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Ultrafast studies of elusive chemical reactions in the gas phase

Dantus

2024

Science

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The chemical composition of the interstellar medium and planetary atmospheres is constantly in flux as atoms and molecules collide and interact with high-energy particles such as electrons, protons, and photons. These transformative processes ultimately lead to the coalescence of molecules and eventually the birth of stars. Our understanding of these chemical ecosystems relies on models that synthesize data from gas-phase experiments, providing insights into reaction cross sections. This Review examines efforts to delve into the fundamental bond-forming and bond-breaking dynamics that occur during bimolecular and electron-initiated reactions. These experiments involve clever approaches to establish a time reference and the collision geometry necessary for tracking atomic motion with femtosecond time resolution. Findings from these efforts enhance present models and improve predictions for molecule-molecule and electron-molecule collisions.

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Ultrafast studies of elusive chemical reactions in the gas phase

Dantus

2024

Science

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scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.

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Unraveling the ultrafast dynamics of thermal-energy chemical reactions

Abstract: In this perspective, we discuss how one can initiate, image, and disentangle the ultrafast elementary steps of thermal-energy chemical dynamics, building upon advances in technology and scientific insight. We propose...

Cited by 1 publication

References 154 publications

Ultrafast studies of elusive chemical reactions in the gas phase

Ultrafast studies of elusive chemical reactions in the gas phase

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