Unveiling the Dynamic Pathways of Metal–Organic Framework Crystallization and Nanoparticle Incorporation for Li–S Batteries
Xiaohui Song,
Rui Huang,
Xingyu Zhang
et al.
Abstract:Metal–organic frameworks (MOFs) present diverse building blocks for high‐performance materials across industries, yet their crystallization mechanisms remain incompletely understood due to gaps in nucleation and growth knowledge. In this study, MOF structural evolution is probed using in situ liquid phase transmission electron microscopy (TEM) and cryo‐TEM, unveiling a blend of classical and nonclassical pathways involving liquid–liquid phase separation, particle attachment–coalescence, and surface layer depos… Show more
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