“…The myriad of defect types and interactions in nuclear fuel under irradiation has motivated researchers to consider improving function by controlling defect evolution and structure. Examples include using dopants to control defect concentrations by modifying grain size [10,11,12,13], simulating HBS using nanocrystalline UO2 to improve fission gas retention and improve mechanical properties [14,15], and directly adding other materials to UO2 to raise the thermal conductivity [16,17,18,19,20,21,22,23,24]. Expediting progress towards tailoring defects and microstructure to bring about desired thermal properties will require further development of fundamental, predictive models of phonon transport in actinide oxide fuels containing irradiation-induced defects [25,26,27,28,29].…”