2024
DOI: 10.1002/anie.202317699
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Using Redox‐Switchable Polymerization Catalysis to Synthesize a Chemically Recyclable Thermoplastic Elastomer

Jiangwei Liu,
Sarah E. Blosch,
Anastasia S. Volokhova
et al.

Abstract: In an effort to synthesize chemically recyclable thermoplastic elastomers, a redox‐switchable catalytic system was developed to synthesize triblock copolymers containing stiff poly(lactic acid) (PLA) end blocks and a flexible poly(tetrahydrofuran‐co‐cyclohexene oxide) (poly(THF‐co‐CHO) copolymer as the mid‐block. The orthogonal reactivity induced by changing the oxidation state of the iron‐based catalyst enabled the synthesis of the triblock copolymers in a single reaction flask from a mixture of monomers. The… Show more

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