Using tannin as a biological curing agent to design fully bio-based epoxidized natural rubber/polylactic thermoplastic vulcanizates with mechanical robustness and multi-stimuli-responsive shape memory properties

Huang, Jiarong; Wu, Haonan; Wang, Xiao; Tan, Lingcao; Xu, Wenhua; Wang, Qiongyao; Liang, Yong; Yu, Huiwen; Liu, Zhan; Xu, Baiping; Xiao, Shuping

doi:10.1016/j.ijbiomac.2024.137173

International Journal of Biological Macromolecules

2024

DOI: 10.1016/j.ijbiomac.2024.137173

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Using tannin as a biological curing agent to design fully bio-based epoxidized natural rubber/polylactic thermoplastic vulcanizates with mechanical robustness and multi-stimuli-responsive shape memory properties

Jiarong Huang,

Haonan Wu,

Xiao Wang

et al.

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Mechanical and Morphological Perspectives on PLA‐Based Thermoplastic Vulcanizates (TPVs): A Brief Review

Shahroodi,

Momeni,

Moshkriz

et al. 2024

Macro Materials & Eng

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Poly(lactic acid) (PLA) brings intriguing prospects to the realm of biodegradable polymers through environmental sustainability, processing, and affordability. However, the widespread use of PLA remains full of challenges mostly because of its brittleness and poor mechanical properties. This review highlighted recent studies on improving PLA brittleness by adding different elastomeric systems and using different crosslinking systems in order to improve the mechanical properties, enhance the interfacial interactions, and stabilize the micromorphology of PLA systems as an effective, promising strategy to mitigate intrinsic PLA problems. Looking at the different microstructures required to achieve better performance, an insightful discussion on the developed morphology between PLA and high‐elastic materials is featured along with reviewing primary mechanical concepts. It concludes with an outlook for static and dynamic vulcanization systems with a perspective of biodegradable PLA and draws attention to the new possibilities that crosslinked PLA can offer.

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Mechanical and Morphological Perspectives on PLA‐Based Thermoplastic Vulcanizates (TPVs): A Brief Review

Shahroodi,

Momeni,

Moshkriz

et al. 2024

Macro Materials & Eng

View full text Add to dashboard Cite

show abstract

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Using tannin as a biological curing agent to design fully bio-based epoxidized natural rubber/polylactic thermoplastic vulcanizates with mechanical robustness and multi-stimuli-responsive shape memory properties

Cited by 1 publication

References 54 publications

Mechanical and Morphological Perspectives on PLA‐Based Thermoplastic Vulcanizates (TPVs): A Brief Review

Mechanical and Morphological Perspectives on PLA‐Based Thermoplastic Vulcanizates (TPVs): A Brief Review

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