Accurate representation of ice accretions is important to the study and understanding of aircraft icing. For research and certification purposes, replicas of ice accretions generated from an icing wind tunnel are created to perform aerodynamic tests in dry-air wind tunnels and in flight. Three-dimensional ice-shape features necessitate aerodynamic observations over the entire surface of the wing or airfoil to fully understand the flow behavior. The pressure-sensitive paint (PSP) technique allows pressure coefficient (C p ) data to be obtained over a larger area and with a greater resolution than is possible by solely using the pressure tap method. Three-dimensional C p measurements obtained as the result of this work both further the understanding of iced-airfoil aerodynamics and provide a validation for a recently developed method of recording ice accretions. Results show the ability of the PSP technique implemented in this experimental study to resolve aerodynamic differences between ice shapes made from the new 3-D ice accretion measurement methodology recently developed by the NASA Icing Research Branch and the current mold and casting method. PSP tests were performed to further investigate the aerodynamics of ice shapes that showed performance variations between the replicas made from the new and current methods. In general, the PSP results agreed with the two-dimensional data obtained from pressure taps while providing additional pressure information along the span. Aerodynamic and PSP agreement between the shapes generated from the two methods was relatively good, but not to the extent expected. Results show the general behaviors agree, with discrepancies in the quantitative data. These discrepancies are shown to be the result of geometric differences in the ice shapes made from the two methods. The 3-D ice accretion measurement methodology was validated for the two tested shapes and possible improvements to the PSP implementation are suggested.