Both regional and localized tectonic events controlled deposition within the Wenlock and early Ludlow of SW Wales. Estuarine deposits within north-south-tending incised valleys dominate the youngest (Homerian) Gray Sandstone Group, valley incision being probably related to changing base-levels associated with Avalonia/Laurentian collision. Available accommodation space was outpaced by sediment supply, with the Red Cliff Formation (Late Ludfordian) defining a conformable transition from marine to Old Red Sandstone (ORS) deposition within the Marloes Peninsula. Sedimentation was dominated by fine-grained pedified siliciclastics, with subordinate fine-grained ephemeral sheet-flood sandstones. Local palaeocurrents indicate sediment transport from the south and west, though long-distance transport from a distant Laurentian provenance is assumed. A probable tectonically generated sequence boundary marks the base of petrographically distinctive, multi-storey pebbly sandstones of the Albion Sands Formation, deposited within the hangingwall valley of the active east-west-trending Wenall Fault. Sediment accommodation space was controlled by proximity to the tip-point of this important growth fault within the Lower ORS. Debris-flow-dominated fans, shed from both the hangingwall and footwall of the Wenall Fault, deposited the Lindsway Bay Formation, an exotic-clast conglomerate unit sourced predominantly from the south and west. It is uncertain as to whether movement along the Wenall Fault was caused by collision-related transtension, or rifting associated with the southern margin of Avalonia.