Variations of Urban NO2 Pollution during the COVID-19 Outbreak and Post-Epidemic Era in China: A Synthesis of Remote Sensing and In Situ Measurements

Abstract

Since the COVID-19 outbreak in 2020, China’s air pollution has been significantly affected by control measures on industrial production and human activities. In this study, we analyzed the temporal variations of NO2 concentrations during the COVID-19 lockdown and post-epidemic era in 11 Chinese megacities by using satellite and ground-based remote sensing as well as in situ measurements. The average satellite tropospheric vertical column density (TVCD) of NO2 by TROPOMI decreased by 39.2–71.93% during the 15 days after Chinese New Year when the lockdown was at its most rigorous compared to that of 2019, while the in situ NO2 concentration measured by China National Environmental Monitoring Centre (CNEMC) decreased by 42.53–69.81% for these cities. Such differences between both measurements were further investigated by using ground-based multi-axis differential optical absorption spectroscopy (MAX-DOAS) remote sensing of NO2 vertical profiles. For instance, in Beijing, MAX-DOAS NO2 showed a decrease of 14.19% (versus 18.63% by in situ) at the ground surface, and 36.24% (versus 36.25% by satellite) for the total tropospheric column. Thus, vertical discrepancies of atmospheric NO2 can largely explain the differences between satellite and in situ NO2 variations. In the post-epidemic era of 2021, satellite NO2 TVCD and in situ NO2 concentrations decreased by 10.42–64.96% and 1.05–34.99% compared to 2019, respectively, possibly related to the reduction of the transportation industry. This study reveals the changes of China’s urban NO2 pollution in the post-epidemic era and indicates that COVID-19 had a profound impact on human social activities and industrial production.

Retrieval of Tropospheric NO2 Vertical Column Densities from Ground-Based MAX-DOAS Measurements in Lhasa, a City on the Tibetan Plateau

“…Due to different lengths of the sunshine duration in different seasons, the longest available time period for MAX-DOAS measurements appeared in July, and the shortest in January. The diurnal variation patterns of tropospheric NO 2 VCDs were different in different seasons, owing to the complex interplay of source emissions, atmospheric photochemical reactions, and dynamic processes [28,35,42,43]. In April and July, the highest tropospheric NO 2 VCDs occurred in the morning and late afternoon with the minimum around 16:00 BJT.…”