Vertical graphene nanowalls supported hybrid W2C/WOx composite material as an efficient non-noble metal electrocatalyst for hydrogen evolution

Rodriguez-Miguel, Shahadev; Ma, Yang; Farid, Ghulam; Amade, Roger; Ospina, Rogelio; Andujar, Jose Luis; Bertran-Serra, Enric; Chaitoglou, Stefanos

doi:10.1016/j.heliyon.2024.e31230

Heliyon

2024

DOI: 10.1016/j.heliyon.2024.e31230

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Vertical graphene nanowalls supported hybrid W2C/WOx composite material as an efficient non-noble metal electrocatalyst for hydrogen evolution

Shahadev Rodriguez-Miguel,

Yang Ma,

Ghulam Farid

et al.

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Cited by 3 publications

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Nanoengineering of CoFe-LDH@Ni(OH)2 for supercapacitor and water splitting applications

Liu,

Zhao,

et al. 2024

J Mater Sci

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Nanoengineering of CoFe-LDH@Ni(OH)2 for supercapacitor and water splitting applications

Liu,

Zhao,

et al. 2024

J Mater Sci

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NdCoO3 nanoparticles grown on reduced graphene oxide sheets as an efficient electrocatalyst for hydrogen evolution reaction

Mahapatra,

Bera,

Kapuria

et al. 2024

International Journal of Hydrogen Energy

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Laser-Induced Vertical Graphene Nanosheets for Electrocatalytic Hydrogen Evolution

Chaitoglou,

Ma,

Ospina

et al. 2024

ACS Appl. Nano Mater.

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Efficient and affordable electrocatalysts are fundamental for the sustainable production of hydrogen from water electrolysis. Here, an approach for the rapid production of laserinduced vertical graphene nanosheets (LIVGNs) through the exfoliation of the graphite foil under laser irradiation is presented. The density of the formed LIVGNs is ∼3 per 100 μm 2 . On leveraging the inherent flexibility and conductivity of the graphite foil substrate, the resulting LIVGNs exhibit a 2.2-fold increase in capacitance, making them promising candidates for electrode applications. The laser-induced surface reconstruction introduces abundant sharp edges to the LIVGNs, enhancing their electrocatalytic potential for hydrogen evolution. In electrocatalytic hydrogen evolution tests in acidic media, the LIVGNs demonstrate superior performance with a remarkable decrease in the required overpotential at 10 mA cm −2 , from −555 mV for the pristine graphite foil to −348 mV for LIVGNs. This improvement is attributed to the active sites provided by the sharp edges, facilitating hydrogen species adsorption. Furthermore, the hydrophilic behavior of LIVGNs is enhanced through the anchoring of oxygencontaining groups, promoting the rapid release of the produced hydrogen bubbles. Importantly, the modified LIVGN electrode exhibits long-term stability across a wide range of current densities during chronoamperometry tests. This research introduces a transformative strategy for the efficient preparation of vertical graphene sheets on conductive graphite foils, showcasing their potential applications in electrocatalysis and energy storage.

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Vertical graphene nanowalls supported hybrid W2C/WOx composite material as an efficient non-noble metal electrocatalyst for hydrogen evolution

Cited by 3 publications

References 43 publications

Nanoengineering of CoFe-LDH@Ni(OH)2 for supercapacitor and water splitting applications

Nanoengineering of CoFe-LDH@Ni(OH)2 for supercapacitor and water splitting applications

NdCoO3 nanoparticles grown on reduced graphene oxide sheets as an efficient electrocatalyst for hydrogen evolution reaction

Laser-Induced Vertical Graphene Nanosheets for Electrocatalytic Hydrogen Evolution

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