Visible-light-promoted and chlorophyll-catalyzed aerobic desulfurization of thioamides to amides

Yang, Zihui; Zhou, Haoyi; Wang, Lin; Zhang, Jingxuan; Xie, Hongfeng; Liu, Yisong; Zeng, Jianguo; Cheng, Pi

doi:10.1039/d2ra01930b

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Radical Precursors Involving C=s Functional Groups1

Organic and Biomolecular Chemistry Review1

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2022

2024

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Cited by 4 publications

(2 citation statements)

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“…While visible light photoredox reactions involving thioketones, thioamides, and benzothioates mainly afforded desulfurization products [67,68] and heterocyclic compounds such as thiazoles [69] and thiadiazoles, [70,71] the current section will highlight the handful of transformations harnessing C=S containing compounds to form C-centered radicals, such as xanthates and Nhydroxy-2-thiopyridones.…”

Section: Radical Precursors Involving C=s Functional Groupsmentioning

confidence: 99%

Sulfur‐Centered Radicals in Visible Light Isocyanide Photochemistry

Russo,

Brunelli,

Tron

et al. 2023

Eur J Org Chem

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Sulfur‐centered radicals have a key role in a plethora of synthetic organic transformations, whose scope has been further expanded thanks to the possibility to generate such species under visible light photocatalytic conditions. The current literature overview focuses on those transformations involving isocyanides and sulfur‐centered radicals with the aim to highlight the chemical space accessible, both in terms of complexity and diversity, and the mechanistic rational underpinning the current and future development of such chemical methodologies.

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Section: Radical Precursors Involving C=s Functional Groupsmentioning

confidence: 99%

Sulfur‐Centered Radicals in Visible Light Isocyanide Photochemistry

Russo,

Brunelli,

Tron

et al. 2023

Eur J Org Chem

View full text Add to dashboard Cite

show abstract

“…Recently, Cheng and co-workers demonstrated the photocatalytic aerobic desulfurization of thioamides under visible light (Scheme 17). 46 The reaction protocol discussed herein provides an environmentally friendly, mild, convenient strategy for the synthesis of amides.…”

Section: Organic and Biomolecular Chemistry Reviewmentioning

confidence: 99%