1995
DOI: 10.1364/ol.20.000878
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Wavelength shifts of dye lasing in microdroplets: effect of absorption change

Abstract: With addition of an absorber to dye-doped microdroplets, an absorption-dependent blue shift in the lasing spectra has been observed. The better the spectral overlap between the absorption and the fluorescence spectra of the dye, the larger the blue shift. The experimental observations are explained by a simple model of dye lasing in an optical cavity that includes losses because of the absorber and radiation leakage.

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Cited by 33 publications
(18 citation statements)
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“…Opposing trends of quality factor and lasing threshold are observed reflecting the interrelated behavior of these quantities. 45 Also consistent with the latter findings is the observation that the gap size influences the spectral position of the WGM lasing. As illustrated in Fig.…”
Section: A Split-disk Micro-cavities-an Alternative Wgm Geometrysupporting
confidence: 71%
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“…Opposing trends of quality factor and lasing threshold are observed reflecting the interrelated behavior of these quantities. 45 Also consistent with the latter findings is the observation that the gap size influences the spectral position of the WGM lasing. As illustrated in Fig.…”
Section: A Split-disk Micro-cavities-an Alternative Wgm Geometrysupporting
confidence: 71%
“…This behavior can again be linked to the change in cavity Q-factor and is a well-understood phenomenon. Such blue shifts are well documented in dye-based micro-lasers for increasing absorption 45 or radiation losses. 32,46,47 In the presented work losses affecting the quality factor are due to the decreasing confinement in the gap region [see Fig.…”
Section: A Split-disk Micro-cavities-an Alternative Wgm Geometrymentioning
confidence: 89%
“…This is accompanied by a decrease of the lasing thresholds due to an increased concentration of dye molecules within the WGMs. These effects can be described by a modified standard dye laser model [11,20], where the number of dye molecules per mode volume depends on the thickness of the gain layer.…”
Section: Lasing In Organic Semiconductor Coated Microgobletsmentioning
confidence: 99%
“…We consider a simple model of dye-lasing. 69,70 We assume that the fluorescentdye molecule can be approximated as a 4-level system. Let rai be the number density (per unit volume) of molecules in the first excited electronic singlet and n 0 be the number density of molecules in the ground electronic singlet state.…”
Section: Dye Lasing In Microdropletsmentioning
confidence: 99%
“…ni<T.(A) > CtleakageW + <Xab,(\, T) + n0<Ta(X), (69) where a; eo t" se is the leakage loss out of the cavity and a a b, is the absorption loss of the liquid and any additive. The absorption and the stimulated emission cross-sections of the dye are <r" and <r e , respectively.…”
Section: Dye Lasing In Microdropletsmentioning
confidence: 99%