2024
DOI: 10.1063/5.0230106
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Wettability regulation of the electric double-layer structural evolution of complex fluids: Insights into thermodynamic and electrical properties

Hongwei Chen,
Yiming Han,
Meng Wang
et al.

Abstract: Understanding the structural evolution at the electrode is essential for accurate prediction of complex fluid applications, where the carbon nanotube is chosen as the carrier of CO2-ionic liquids (ILs) in electroreduction. Then, the electrical double layer with tunable wettability is investigated by molecular dynamics simulations. The competition and cooperation between van der Waals and Coulomb interactions are evaluated by examining the structural and electric characteristics. When an external potential (φ) … Show more

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