Soldiers and supporting engineers are frequently exposed to high low-frequency (<500 Hz) cabin noise in military vehicles. Despite the use of commercial hearing protection devices, the risk of auditory damage is still imminent because the devices may not be optimally customised for such applications. This study considers flax fibre-reinforced polypropylene (Flax-PP) as an alternative to the material selection for the ear cups of commercial earmuffs, which are typically made of acrylonitrile butadiene styrene (ABS). Different weaving configurations (woven and nonwoven) and various noise environments (pink noise, cabin booming noise, and firing noise) were considered to investigate the feasibility of the proposed composite earmuffs for low-frequency noise reduction. The remaining assembly components of the earmuff were kept consistent with those of a commercial earmuff, which served as a benchmark for results comparison. In contrast to the commercial earmuff, the composite earmuffs were shown to be better in mitigating low-frequency noise by up to 16.6 dB, while compromising midfrequency acoustical performance. Consequently, the proposed composite earmuffs may be an alternative for low-frequency noise reduction in vehicle cabins, at airports, and at construction sites involving heavy machineries.