“…Recently, considerable research has been conducted on borate series nonlinear optical crystals for harmonic generation in high-power solid-state ultraviolet (UV) lasers due to their excellent properties such as relatively high tolerance to laser-induced damage, large nonlinear optical coefficients, moderate birefringence, and wide transparency range in the UV region. For instance, several borate crystals, such as β-BaB 2 O 4 (BBO) [4], LiB 3 O 5 (LBO) [5], CsB 3 O 5 (CBO) [6], CsLiB 6 O 10 (CLBO) [7,8], KBe 2 BO 3 F 2 (KBBF) [9], YCa 4 O(BO 3 ) 3 (YCOB) [10], and YA1 3 (BO) 4 (YAB) [11] have attracted a great deal of attention. Among these crystals, CLBO is a newly developed borate crystal and has been successfully applied for the fourth and fifth-harmonic generation of a Nd:YAG laser [12,13].…”