Magnesium-calcium alloy composites reinforced with nickel-coated vapor-grown carbon bers (VGCFs) were fabricated using a compo-casting process. Then, the microstructures and mechanical properties of these composites were investigated. The Mg-5Al-3Ca (AX53) alloy exhibited a dendritic microstructure with a coarse lamellar (Mg, Al) 2 Ca phase along the grain boundaries instead of the irregular β-Mg 17 Al 12 phase found in the Mg-5Al alloy. For the 0.5% Ni-coated VGCF-reinforced AX53 alloy composite, the VGCFs were well dispersed in the matrix, with the nickel coating diffused into the metal. Al 3 Ni compounds formed both inside the grains and on the grain boundaries. The ultimate tensile strength (UTS) and strain-hardening of the AX53 alloy, in comparison with the Mg-5Al alloy, were improved signi cantly to the point of fracture. Furthermore, an increase in the UTS of the composite was achieved with the addition of 0.5% VGCFs, along with an increase in the total elongation, which could mainly be attributed to the strain hardening during a larger strain. The 0.2% yield stress was slightly improved as a result of the small amount of introduced Ni-coated VGCFs. However, the elongation dropped for the 1.0% VGCF-reinforced AX53 alloy composites, which led to a low strength similar with that of the AX53 alloy.