quasiparticles as Majorana-bound states (MBS) that demonstrate non-Abelian statistics which can be used for topological quantum computation applications. [1,2] There are several possible avenues for creating topological superconductivity which hosts MBS. [3] For example, these MBS can be realized on the boundary of a superconductor with an intrinsic oddparity, for example, spin-triplet or p-wave, pairing state. [3,4] However, only a few candidate p-wave superconductors exist, such as Cu x Bi 2 Se 3 and UTe 2 , which tend to have a low superconducting transition temperature (T c ) and are sensitive to disorder. [5][6][7][8][9][10][11] Another example is nanowire heterojunctions between semiconducting and superconducting materials with large spin-orbit coupling which can host MBS at the ends of the wires when placed in a magnetic field. [12,13] Unfortunately, the existence of MBS in these systems is also sensitive to uniformity arising from materials and device fabrication processes. [14] Finally, there are several avenues to create MBS via topological superconductivity from proximity-induced effects. [3] Prominent examples include superconducting materials with topological surface states and the interface between a s-wave superconductor and a topological insulator (TI), where the superconducting proximity effect induces an effective p-wave pairing in the TIS . [3,15] Among this class of candidate topological superconductors, the Fe(Te,Se) system has attracted considerable attention. [16][17][18][19][20][21][22][23][24] Both FeTe and FeSe, as well as the alloyed Fe(Te,Se) system, have an electronic band structure that is related to the ironpnictide family of high-T c superconductors. [18,[25][26][27] In general, the Fermi surfaces are dominated by bands derived from the Fe d-orbitals that result in hole pockets at the Brillouin zone center (Γ) and electron pockets at the zone boundary (M). First principles calculations for the two parent compounds reveal FeTe to have a larger Fermi surface and larger density of states at the Fermi level compared to FeSe. [25] These differences are due to subtle changes in the band shapes and relative energies arising from height differences between Se/Te and the Fe plane. As the two materials are alloyed, the Fe(Te,Se) system reveals spin-helical Dirac surface states due to the topological band inversion between the p z and d xy /d yz bands as the p z bandThe interface between 2D topological Dirac states and an s-wave superconductor is expected to support Majorana-bound states (MBS) that can be used for quantum computing applications. Realizing these novel states of matter and their applications requires control over superconductivity and spin-orbit coupling to achieve spin-momentum-locked topological interface states (TIS) which are simultaneously superconducting. While signatures of MBS have been observed in the magnetic vortex cores of bulk FeTe 0.55 Se 0.45 , inhomogeneity and disorder from doping make these signatures unclear and inconsistent between vortices. Here superconduc...