We demonstrate in an optical fiber that third-order dispersion yields an unexpected symmetry-breaking dynamics of the modulational instability spectrum. It is found in particular that this spectral asymmetry does not smoothly and monotonically increase when approaching the zero-dispersion wavelength. Instead, it exhibits several local extrema and it can even be reversed at a particular dispersion value. We interpret this behavior as resulting from interactions between dispersive waves and solitons generated from modulation instability.
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