A computational model for the optimization of the second order optical nonlinearities in GaInAs/AlInAs quantum cascade laser structures is presented. The set of structure parameters that lead to improved device performance was obtained through the implementation of the Genetic Algorithm. In the following step, the linear and second harmonic generation power were calculated by self-consistently solving the system of rate equations for carriers and photons. This rate equation system included both stimulated and simultaneous double photon absorption processes that occur between the levels relevant for second harmonic generation, and material-dependent effective mass, as well as band nonparabolicity, were taken into account. The developed method is general, in the sense that it can be applied to any higher order effect, which requires the photon density equation to be included. Specifically, we have addressed the optimization of the active region of a double quantum well In 0.53 Ga 0.47 As/Al 0.48 In 0.52 As structure and presented its output characteristics. V C 2014 AIP Publishing LLC. [http://dx

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We report on experimental observation of low-threshold Risken-Nummedal-Graham-Haken (RNGH) instability in mid-infrared InGaAs/InAlAs Quantum Cascade Lasers (QCLs) operating at 8 µm wavelength. The devices employ sequential resonant tunneling and can provide optical gain on the diagonal or vertical transition. Depending on the tunneling resonance detuning, the lasers can operate either on a stable part of I-V curve or with unstable electric field domain formation. We report how all these features impact the occurrence of the RNGH instability with broadband multimode emission, and show how they can be tailored with an applied bias or via optical excitation of free carriers. We present the results of 2 nd order interferometric autocorrelation measurements and time-resolved spectral measurements in free-running QCLs and QCLs subjected to optical pumping. We explain the diversity of dynamic regimes in QCLs using a simple analytical expression for the second threshold.