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A field investigation was conducted to evaluate the effectiveness of store-and-release (SR) covers made with different phosphate mine wastes in reducing water infiltration (system inclination and surface runoff were neglected) and controlling acid rock drainage (ARD) generation. Four instrumented experimental cells were constructed with different SR layer configurations (two thicknesses and three materials) placed over a capillary break layer. To assess the hydrogeological behaviour of these cover systems, volumetric water content, matric suction, and meteorological monitoring time trends were studied for a period of 1.5 years under actual and extreme conditions typical of an arid climate. Under natural climatic conditions, all net infiltration was released to the atmosphere by the physical process of evaporation (regardless of SR layer thickness and type). Although high surface matric suction (>3000 kPa) decreased the evaporation rate (or release capacity) during the drying period, field tests showed that the studied scenarios limited deep water infiltration even under extreme rainfall events. The release capacity of the SR layer was slightly lower for cover systems made with the finer-grained mine waste (phosphate limestone tailings). This study showed that, for a one-dimensional (1D) condition, the tested phosphate mine wastes have the appropriate hydrogeological properties to be used as components of SR covers under conditions at the Kettara mine site, located near Marrakech, Morocco.