To overcome a bottleneck in spintronic applications such as those of ultralow-power magnetoresistive random-access memory devices, the electric-field control of magnetization vectors in ferromagnetic electrodes has shown much promise. Here, we show the giant converse magnetoelectric (CME) effect in a multiferroic heterostructure consisting of the ferromagnetic Heusler alloy Co2FeSi and ferroelectric-oxide Pb(Mg1/3Nb2/3)O3-PbTiO3 (PMN-PT) for electric-field control of magnetization vectors. Using an in-plane uniaxial magnetic anisotropy of polycrystalline Co2FeSi film grown on PMN-PT(011), the nonvolatile and repeatable magnetization vector switchings in remanent states are demonstrated. The CME coupling coefficient of the polycrystalline Co2FeSi/PMN-PT(011) is over 1.0 × 10−5 s/m at room temperature, comparable to those of single-crystalline Fe1-xGax/PMN-PT systems. The giant CME effect has been demonstrated by the strain-induced variation in the magnetic anisotropy energy of Co2FeSi with an L21-ordered structure. This approach can lead to a new solution to the reduction in the write power in spintronic memory architectures at room temperature.
A structural and FMR study is presented for epitaxial thin films of the Heusler alloy Co 2 FeAl 0.5 Si 0.5 (CFAS) grown on Ge(111) and Si(111) substrates. All films, as-grown and post-annealed, show B2 ordering; full chemical order (L2 1 ) is not obtained over the range of anneal temperatures used in this study. As-grown films show a lower Gilbert damping constant, a, when grown on a Si(111) substrate compared to Ge(111). Annealing the films to 450 C significantly reduces a for CFAS on Ge while increasing a for CFAS on Si. This is related to a substrate dependent competition between improvements in lattice structure and increased interfacial intermixing as a function of anneal temperature. The optimal annealing temperature to minimize a is found to differ by $100 K between the two substrates. Above an anneal temperature of 500 C, films grown on both substrates have increased coercivity, decreased saturation magnetization, and show characteristic two-magnon scattering features.
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