The scheme of a generation of ultrasound waves based on optically excited Tamm plasmon structures is proposed. It is shown that Tamm plasmon structures can provide total absorption of a laser pulse with arbitrary wavelength in a metallic layer providing the possibility of the use of an infrared semiconductor laser for the excitation of ultrasound waves. Laser pulse absorption, heat transfer and dynamical properties of the structure are modeled, and the optimal design of the structure is found. It is demonstrated that the Tamm plasmon-based photoacoustic generator can emit ultrasound waves in the frequency band up to 100 MHz with predefined frequency spectrum.
The properties of the ultrastrongly coupled Tamm plasmon cavity filled with a high-oscillator-strength organic material DPAVBi (4,4′-bis[4-(di-ptolylamino)styryl]biphenyl) are studied using theoretical and experimental methods. An analytical model predicts the opposite sign of polarization splitting for the lower and upper polariton cases and a giant absolute value of the splitting. A set of organic Tamm plasmon cavities with different detuning parameters are fabricated. We demonstrate that all structures are operating in the ultrastrong coupling regime: the values of the Rabi splitting are close to a 20% fraction of the exciton energy. The measured angle-dependent reflectivity spectra structure for both transverse electric (TE) and transverse magnetic (TM) polarizations confirm the predicted theoretical model. We obtained a giant value of the polarization splitting of up to 180 meV for both polariton branches. We believe that it is the first demonstration of such peculiar polarization splitting behavior of polaritons in the ultrastrong coupling regime.
Excitons in organic semiconductors possessing a large oscillator strength demonstrate strong coupling with cavity modes at room temperature. A large Stokes shift in some organic semiconductors enriches and complicates the picture of the emission in strongly coupled systems of organic excitons and light. Here we demonstrate strong coupling of excitons in 4,4-Bis(N-carbazolyl)-1,1-biphenyl (CBP) and Tamm plasmons in the UV band, accompanied by a bright emission from the structure. Reflection measurements demonstrate the pronounced formation of the lower and upper polariton modes with Rabi splitting of the magnitude of 0.3 eV, and the emission peak experiences a substantial red shift with respect to the lower polariton mode. Both radiative and nonradiative decay rates in the Tamm plasmon CBP structure are increased with respect to a bare CBP. Such peculiar behavior is attributed to the simultaneous manifestation of strong coupling and weak coupling of the CBP molecule emitters to the Tamm plasmons.
Control of directionality of emissions is an important task for the realization of novel nanophotonic devices based on nanowires. Most of the existing approaches providing high directionality of the light emitted from nanowires are based on the utilization of the tapered shape of nanowires, serving as nanoantenna coupling with the light waveguided in nanowire and the directional output beam. Here we report the beaming of the emitted light with wavelength near 800 nm by naturally formed core-shell AlGaAs NW with multiply GaAs quantum dots (QDs) diameter 30 nm and height 10 nm, while the diameter of NW 130 nm, what does not support efficient emission into waveguided modes, including the mode HE11. Experimental measurements show that intensity of emission for directions in the vicinity of the axis of NW is about two orders of magnitude higher than for perpendicular directions. The developed theoretical approach allowed us to calculate the probability of spontaneous emission for various directions and into waveguided modes and showed that highly directional radiation can be provided by the intrinsic emission properties of cylindrical NW. Our results suggest that for the small diameter of NW, directional emissions are associated with an TM0 leaky mode (when electric field oriented in axial direction) and therefore manifests in an existence of axial electric dipole transitions in quantum dots.
The interaction of an exciton and cavity modes is considered in planar meso-cavities, which have lateral sizes corresponding to few wavelengths. In meso-cavities, the frequency interval between the optical modes is comparable or smaller than the value of the Rabi splitting between the exciton and the optical modes. The Hamiltonian of the interaction between the exciton and the cavity modes is constructed, and it is shown that such an interaction between the cavity modes and the exciton can occur both in weak and in strong coupling regimes. The latter case can be accompanied by a pronounced splitting of the emission peaks as shown for modelled meso-cavities of triangular, square and hexagonal shapes, where it is demonstrated that Q-factors for the adjacent cavity modes as well as the strength of interaction with excitons can differ by few orders of magnitude.
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