We describe an interferometric technique suitable for determination of piezo-optic coefficients (POCs) in crystals. The method considers real nonparallelism of measured samples, thereby improving the measuring precision of POCs significantly. Corresponding equations are derived for the interferometric half-wave stress method. Using this technique we have determined a complete set of POCs of pure and MgO-doped LiNbO(3) crystals. The reliability of the data has been confirmed by comparing the effective POCs expressed through the combinations of measured POCs and the effective POCs determined independently using highly precise optical birefringence measurements. Pure and MgO-doped LiNbO(3) crystals reveal nearly the same magnitudes of POCs. However, LiNbO(3):MgO exhibits about 4 times higher resistance with respect to powerful light radiation, making it more suitable for application in acousto-optic devices that deal with superpowerful laser radiation.

This paper presents the results of ultrasonic measurements of LiNbO 3 and LiNbO 3 : MgO crystals. The tensors of piezoelectric coefficients, elastic stiffness constants, and elastic compliances are determined for both crystals at room temperature. Combining these data with the results of piezo-optical measurements, a complete set of photoelastic tensor coefficients is also calculated. Doping of LiNbO 3 crystals by MgO does not lead to a considerable modification of their elastic and photoelastic properties. However, LiNbO 3 : MgO is characterized by a considerably higher resistance with respect to powerful light radiation, making it promising for future application in acousto-optic devices that deal with superpowerful laser radiation. Presented here are the complete tensor sets of elastic constants and photoelastic coefficients of LiNbO 3 and LiNbO 3 : MgO crystals that may be used for a geometry optimization of acousto-optical interaction providing the best diffraction efficiency of acousto-optical cells made of these materials.

We suggest a method for optimizing geometry of acousto-optic (AO) interactions in anisotropic crystalline materials. Within the framework of this method, one gets global maximums of AO figure of merit M2 and their spatial orientations, proceeding from so-called “extreme” indicative surfaces, which are obtained after finding such an acoustic wave propagation direction that maximizes the M2 parameter for each propagation direction of the incident electromagnetic wave. The method improves earlier indicative surface-based techniques in several aspects, particularly in properly accounting for the momentum conservation condition for the AO diffraction, and yields a higher accuracy in assessing spatial anisotropy of the AO effect. We have constructed the extreme surfaces of LiNbO3 crystals for all possible cases, including those of isotropic/anisotropic AO diffractions and longitudinal/transverse acoustic waves. The anisotropy of the AO figure of merit for LiNbO3 is analyzed for the acoustic frequencies 0.01–2.0 GHz and the light wavelengths 405–1444 nm. The absolute M2 maximums refer to ‘indirect crystal cuts' and are equal to 26.3 × 10−15 s3/kg at 2 GHz and 405 nm, and 15.4 × 10−15 s3/kg at 0.4 GHz and 1444 nm.

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