Understanding the evolution of spin-orbit torque (SOT) with increasing heavy-metal thickness in ferromagnet/normal metal (FM/NM) bilayers is critical for the development of magnetic memory based on SOT. However, several experiments have revealed an apparent discrepancy between damping enhancement and damping-like SOT regarding their dependence on NM thickness. Here, using linewidth and phase-resolved amplitude analysis of vector network analyzer ferromagnetic resonance (VNA-FMR) measurements, we simultaneously extract damping enhancement and both field-like and damping-like inverse SOT in Ni 80 Fe 20 /Pt bilayers as a function of Pt thickness. By enforcing an interpretation of the data which satisfies Onsager reciprocity, we find that both the damping enhancement and damping-like inverse SOT can be described by a single spin diffusion length (≈ 4 nm), and that we can separate the spin pumping and spin memory loss contributions to the total damping. This analysis indicates that less than 40% of the angular momentum pumped by FMR through the Ni 80 Fe 20 /Pt interface is transported as spin current into the Pt. On account of the spin memory loss and corresponding reduction in total spin current available for spin-charge transduction in the Pt, we determine the Pt spin Hall conductivity (σ SH = (2.36 ± 0.04) × 10 6 Ω −1 m −1 ) and bulk spin Hall angle (θ SH = 0.387 ± 0.008) to be larger than commonly-cited values. These results suggest that Pt can be an extremely useful source of SOT if the FM/NM interface can be engineered to minimize spin loss. Lastly, we find that self-consistent fitting of the damping and SOT data is best achieved by a model with Elliott-Yafet spin relaxation and extrinsic inverse spin Hall effect, such that both the spin diffusion length and spin Hall conductivity are proportional to the Pt charge conductivity. * thomas.silva@nist.gov † Contribution of the National Institute of Standards and Technology; not subject to copyright.

We report the manipulation of nitrogen vacancy (NV) spins in diamond when nearby ferrimagnetic insulator, yttrium iron garnet, is driven into precession. The change in NV spin polarization, as measured by changes in photoluminescence, is comparable in magnitude to that from conventional optically detected magnetic resonance, but relies on a distinct mechanism as it occurs at a microwave frequency far removed from the magnetic resonance frequency of the NV spin. This observation presents a new approach to transferring ferromagnetic spin information into a paramagnet and then transducing the response into a robust optical signal. It also opens new avenues for studying ferromagnetism and spin transport at the nanoscale.

Functional spintronic devices rely on spin-charge interconversion effects, such as the reciprocal processes of electric field-driven spin torque and magnetization dynamics-driven spin and charge flow. Both damping-like and field-like spin-orbit torques have been observed in the forward process of current-driven spin torque and damping-like inverse spin-orbit torque has been well-studied via spin pumping into heavy metal layers. Here we demonstrate that established microwave transmission spectroscopy of ferromagnet/normal metal bilayers under ferromagnetic resonance can be used to inductively detect the AC charge currents driven by the inverse spin-charge conversion processes. This technique relies on vector network analyzer ferromagnetic resonance (VNA-FMR) measurements. We show that in addition to the commonly-extracted spectroscopic information, VNA-FMR measurements can be used to quantify the magnitude and phase of all AC charge currents in the sample, including those due to spin pumping and spin-charge conversion. Our findings reveal that Ni80Fe20/Pt bilayers exhibit both damping-like and field-like inverse spin-orbit torques. While the magnitudes of both the damping-like and field-like inverse spin-orbit torque are of comparable scale to prior reported values for similar material systems, we observed a significant dependence of the damping-like magnitude on the order of deposition. This suggests interface quality plays an important role in the overall strength of the damping-like spin-to-charge conversion.