No abstract

Plasmonic nanopatch antennas that incorporate dielectric gaps hundreds of picometers to several nanometers thick have drawn increasing attention over the past decade because they confine electromagnetic fields to grossly sub-diffraction-limited volumes. Substantial control over the optical properties of excitons and color centers confined within these plasmonic cavities has already been demonstrated with far-field optical spectroscopies, but near-field optical spectroscopies are essential for an improved understanding of the plasmon–emitter interaction at the nanoscale. Here, we characterize the intensity and phase-resolved plasmonic response of isolated nanopatch antennas by cathodoluminescence microscopy. Furthermore, we explore the distinction between optical and electron beam spectroscopies of coupled plasmon–exciton heterostructures to identify constraints and opportunities for future nanoscale characterization and control of hybrid nanophotonic structures. While we observe substantial Purcell enhancement in time-resolved photoluminescence spectroscopies, negligible Purcell enhancement is observed in cathodoluminescence spectroscopies of hybrid nanophotonic structures. The substantial differences in measured Purcell enhancement for electron beam and laser excitation can be understood as a result of the different selection rules for these complementary experiments. These results provide a fundamentally new understanding of near-field plasmon–exciton interactions in nanopatch antennas, which is essential for myriad emerging quantum photonic devices.

Nonreciprocal thermal emission is a cutting-edge technology that enables fundamental control over thermal radiation and has exciting applications in thermal energy harvesting. However, thus far one of the foremost challenges is making nonreciprocal emission operate over a broad wavelength range and for multiple angles. In this work, we solve this outstanding problem by proposing three different types of structures that always utilize only one Weyl semimetal (WSM) thin film combined with one or two additional dielectric or metallic layers and terminated by a metallic substrate. First, a tradeoff relationship between the magnitude and bandwidth of the thermal nonreciprocity contrast is established based on the thickness of the WSM film. Then, the bandwidth broadening effect is demonstrated via the insertion of a dielectric spacer layer that can also be fine-tuned by varying its thickness. Finally, further control on the resulting strong nonreciprocal thermal radiation is demonstrated by the addition of a thin metallic layer in the proposed few layer designs. The presented composite structures work for a broad frequency range and for multiple emission angles, resulting in highly advantageous properties for various nonreciprocal thermal radiation applications. Moreover, the proposed designs do not require any patterning and can be experimentally realized by simple deposition fabrication methods. They are expected to aid in the creation of broadband nonreciprocal thermal emitters that can find applications in new energy harvesting devices.

Controlling the spectral and angular response of infrared (IR) radiation is a challenging task of paramount importance to various emerging photonic applications. Here, we overcome these problems by proposing and analyzing a new design of a tunable narrowband directional optical transmission filter. The presented thermally controlled multilayer filter leverages the temperature dependent phase change properties of vanadium dioxide (VO2) to enable efficient and reversible fast optical switching by using a pump-probe laser excitation setup. More specifically, transmission is blocked for high intensity probe lasers due to the VO2 metallic properties induced at elevated temperatures while at low probe laser intensities high transmission through the filter occurs only for a narrowband IR range confined to near normal incident angles. The proposed multilayer composite dielectric filter is expected to have applications in optical communications, where it can act as dual functional infrared filter and optical switch.

Surfaces with high directional electromagnetic absorption or emission in the infrared (IR) region of the electromagnetic spectrum have numerous potential applications, however many of the relevant surfaces suffer from extremely narrow bandwidth and/or polarization dependence. Here we demonstrate broadband directional emissivity in the mid-infrared range of 7.5 to 14 µm, that is not dependent on polarization. This was achieved with angled micro-scale structures that are overlaid with nano-scale features on stainless steel 304 produced using an emerging fabrication technique known as femtosecond laser surface processing (FLSP). FLSP is an advanced surface functionalization technique that produces hierarchical micro-and nano-scale quasi-periodic surface features in a single laser processing step. Here we report a surface with peak emission for an angle of 55° using FLSP to create fin-shaped micro-and nano-scale surface features that are tilted at a 55° angle. Cross sectioning of the fin-shaped structures using focused ion beam milling was performed to understand the morphology and subsurface microstructure. Cross-sectional images and energy dispersive X-ray spectroscopy analysis show the structure consists of a thin redeposited oxide layer and the bulk of the fin structure is consistent with the original stainless-steel alloy. The emission results are verified by full-wave electromagnetic simulations which consider all the diffraction-orders performed utilizing the finite element method software, COMSOL Multiphysics, that predicts with reasonable accuracy the resulting directional emissivity of the laser processed surface.