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This work presents betanin dye-loaded TiO2-ZnO thin film solar cells for solar energy harvesting. The TiO2-ZnO nanocomposite was prepared by the one-step microwave-assisted technique. Structural studies exhibit mixed phases of rutile and wurtzite structure of TiO2 and ZnO respectively. The morphological investigations of deposited TiO2-ZnO nanocomposite showed interconnected many-fold nanoflakes morphology. EDS confirms the formation of stoichiometric TiO2-ZnO nanocomposite films. An optical study demonstrates electronic transition with a bandgap energy range of 2.72 to 2.94eV. Photovoltaic performance shows photocurrent from 1.62 to 2.73 mA/cm2 with the photovoltage of 659-795 mV in the range with a 3.25 % photo-conversion efficiency for the sample of TZO3 dye-sensitized solar cell (DSSCs).