Abstract. Metastability exchange optical pumping (MEOP) is experimentally investigated in3 He at 4.7 T, at room temperature and for gas pressures ranging from 1 to 267 mbar. The 2 3 S-2 3 P transition at 1083 nm is used for optical pumping and for detection of the laser-induced orientation of 3 He atoms in the rf discharge plasma. The collisional broadening rate is measured (12.0 ± 0.4 MHz mbar −1 FHWM) and taken into account for accurate absorption-based measurements of both nuclear polarization in the ground state and atom number density in the metastable 2 3 S state. The results lay the ground for a comprehensive assessment of the efficiency of MEOP, by comparison with achievements at lower field (1 mT-2 T) over an extended range of operating conditions. Stronger hyperfine decoupling in the optically pumped 2 3 S state is observed to systematically lead to slower build-up of 3 He orientation in the ground state, as expected. The nuclear polarizations obtained at 4.7 T still decrease at high pressure but in a less dramatic way than observed at 2 T in the same sealed glass cells. To date, thanks to the linear increase in gas density, they correspond to the highest nuclear magnetizations achieved by MEOP in pure 3 He gas. The improved efficiency puts less demanding requirements for compression stages in polarized gas production systems and makes high-field MEOP particularly attractive for magnetic resonance imaging of the lungs, for instance.
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