We present experimental measurements of the normal stresses in sheared Stokesian suspensions. Though the suspending fluid is Newtonian, dispersing rigid non-Brownian particles in it yields a suspension that is non-Newtonian, as it exhibits normal stress differences and an excess isotropic pressure in viscometric flows. At small to moderate concentrations, the normal stresses are very small in magnitude, and hence difficult to measure. This difficulty is compounded by the presence of noise due to unavoidable experimental artifacts. Owing to these limitations, most measurements reported earlier were carried out at relatively high particle concentrations, and some at shear rates large enough that the effects of particle and fluid inertia may have been significant. In our study, we have used a novel technique to measure the small stress levels. This was achieved by applying a sinusoidally varying shear rate with a fixed (low) frequency superimposed on a constant shear rate, and using a lock-in amplifier to measure the Fourier component of the same frequency in the stress signal. We have measured normal stresses in cylindrical-Couette and parallel-plate geometries, and combined these measurements to determine the two normal stress differences for particle volume fractions in the range 0.3–0.45. While the normal stresses are very small at low concentrations, they rise rapidly with increasing concentration. The normal stresses vary linearly with the magnitude of the shear rate, and are independent of its sign. In contrast to polymeric solutions, both normal stress differences are negative, and the first normal stress difference is significantly smaller in magnitude. We compare our data with the results of earlier studies, and observe good agreement.

We report the normal stresses in a non-Brownian suspension in plane Couette flow determined from Stokesian Dynamics simulations. The presence of normal stresses that are linear in the shear rate in a viscometric flow indicates a non-Newtonian character of the suspension, which is otherwise Newtonian. While in itself of interest, this phenomenon is also important because it is believed that normal stresses determine the migration of particles in flows with inhomogeneous shear fields. We simulate plane Couette flow by placing a layer of clear fluid adjacent to one wall in the master cell, which is then replicated periodically. From a combination of the traceless hydrodynamic stresslet on the suspended particles, the stresslet due to (non-hydrodynamic) inter-particle forces, and the total normal force on the walls, we determine the hydrodynamic and inter-particle force contributions to the isotropic ‘particle pressure’ and the first normal stress difference. We determine the stresses for a range of the particle concentration and the Couette gap. The particle pressure and the first normal stress difference exhibit a monotonic increase with the mean particle volume fraction ϕ. The ratio of normal to shear stresses on the walls also increases with ϕ, substantiating the result of Nott & Brady (1994) that this condition is required for stability to concentration fluctuations. We also study the microstructure by extracting the pair distribution function from our simulations; our results are in agreement with previous studies showing anisotropy in the pair distribution, which is the cause of normal stresses.

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