Monitoring of environmental radiation helps to ascertain healthy vicinity which is a catalyst to the economic development of the area. Activity concentration of naturally occurring radionuclides in three (3) dumpsites in Lagos State, Olusosun Landfill, Ojota, Ilupeju dumpsite and, Gbagada dumpsite Lagos state, Nigeria were investigated using gamma-ray spectroscopy to obtain the level of radioactive exposure hazards experienced by people living in these vicinities. A total of thirty soil samples were randomly collected into a polythene bag. They were oven-dried at 110°C, pulverized, and sieved. Quantities of the samples (400 g) were sealed in cylindrical sample holders and kept for about 28 days to attain secular equilibrium between 226Ra and its decay products before analysis using gamma-ray spectrometry. The mean activity concentration obtained for 40K, 238U, and 234Th at, Ilupeju, Gbagada, and Ojota were 339.23±33.66, 11.83±19.174, 11.95±22.752 Bq/kg, 337.56 ± 36.22, 11.49±22.14, 11.54 ± 19.33 Bq/kg and 334.87±32.44, 11.42±22.39, 11.56±18.52 Bq/kg respectively. The mean absorbed dose nGy/h, annual effective dose mSv/y were calculated and their results were found to be below the global values. The results indicate that the radiation level within the dumpsites poses no significant health risk to the people living close to the dumpsites.
Qualitative analysis of radionuclides requires the use of reliable gamma-ray detection system. The NaI(Tl) detector has been widely used and still one of the most used detectors today. It is therefore imperative to validate the reliability of the 5x5 cm2 NaI(Tl) gamma spectrometry system used in carrying out gamma-ray analysis of soil samples in the Radiation and Health Laboratory, Federal University of Agriculture Abeokuta, Nigeria. The gamma ray spectrometer is housed in a 5 cm thick cylindrical lead shield. Calibration was executed using standard materials produced under the auspices of the International Atomic Energy Agency (IAEA). Resolution and detection limit (LD) of the detector were determined using full width at half the maximum of the energy peak of 137Cs and background signal level of the reference materials respectively. Counting efficiencies of the detector was calculated using energies of 1460 keV, 1764keV and 2615 keV for 40K, 226Ra and 232Th respectively. Secondary samples, RGMIX1 and RGMIX2 were formulated and counted to calculate activity concentrations using the NaI(Tl) detector. Resolution of the detector was calculated to be 7.8% of 137Cs, which is good for a NaI(Tl) detector. The counting efficiency of the detector is seen to depend on the gamma ray energy. The results from this work shows that the detector system is suitable gamma spectrometry, and will give quality measurements when used for quantitative determination of radionuclides in environmental samples. The efficiency and resolution of the NaI(Tl) detector should also be determined using photon energies obtained from other radioactive sources.
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