Abstract. On April 15 and 19, 1998, two intense dust storms were generated over the Gobi desert by springtime low-pressure systems descending from the northwest. The windblown dust was detected and its evolution followed by its yellow color on SeaWiFS satellite images, routine surface-based monitoring, and through serendipitous observations. The April 15 dust cloud was recirculating, and it was removed by a precipitating weather system over east Asia

Smog chamber experiments were conducted to investigate the chemical and physical transformations of organic aerosol (OA) during photo-oxidation of open biomass burning emissions. The experiments were carried out at the US Forest Service Fire Science Laboratory as part of the third Fire Lab at Missoula Experiment (FLAME III). We investigated emissions from 12 different fuels commonly burned in North American wildfires. The experiments feature atmospheric and plume aerosol and oxidant concentrations; aging times ranged from 3 to 4.5 h. OA production, expressed as a mass enhancement ratio (ratio of OA to primary OA (POA) mass), was highly variable. OA mass enhancement ratios ranged from 2.9 in experiments where secondary OA (SOA) production nearly tripled the POA concentration to 0.7 in experiments where photo-oxidation resulted in a 30 % loss of the OA mass. The campaign-average OA mass enhancement ratio was 1.7 ± 0.7 (mean ± 1σ); therefore, on average, there was substantial SOA production. In every experiment, the OA was chemically transformed. Even in experiments with net loss of OA mass, the OA became increasingly oxygenated and less volatile with aging, indicating that photo-oxidation transformed the POA emissions. Levoglucosan concentrations were also substantially reduced with photo-oxidation. The transformations of POA were extensive; using levoglucosan as a tracer for POA, unreacted POA only contributed 17 % of the campaign-average OA mass after 3.5 h of exposure to typical atmospheric hydroxyl radical (OH) levels. Heterogeneous reactions with OH could account for less than half of this transformation, implying that the coupled gas-particle partitioning and reaction of semi-volatile vapors is an important and potentially dominant mechanism for POA processing. Overall, the results illustrate that biomass burning emissions are subject to extensive chemical processing in the atmosphere, and the timescale for these transformations is rapid

In the spring of 1985 an interagency consortium of federal land management agencies and the Environmental Protection Agency established the Interagency Monitoring of Protected Visual Environments (IMPROVE) network to assess visibility and aerosol monitoring for the purpose of tracking spatial and temporal trends of visibility and visibility‐impairing particles in rural areas. The program was initiated with 20 monitoring sites and was expanded to 165 sites between 2000 and 2003. This paper reports on fine aerosol data collected in the year 2001 at 143 sites. The major fine (dp < 2.5 μm) particle aerosol species, sulfates, nitrates, organics, light‐absorbing carbon, and wind‐blown dust, and coarse gravimetric mass are monitored, and at some sites, light scattering and/or extinction are measured. Sulfates, carbon, and crustal material are responsible for most of the fine mass at the majority of locations throughout the United States, while at sites in southern California and the midwestern United States, nitrates can contribute significantly. In the eastern United States, sulfates contribute between 50 and 60% of the fine mass. Sulfate concentrations tend to be highest in the summer months while organic concentrations can be high in the spring, summer, or fall seasons, depending upon fire‐related emissions. However, at the two urban sites, Phoenix, Arizona, and Puget Sound, Washington, organics peak during the winter months. Nitrate concentrations also tend to be highest during the winter months. During the spring months in many areas of the western United States, fine soil can contribute as much as 40% of fine mass. The temporal changes in soil concentration that occur simultaneously over much of the western United States including the Rocky Mountain region suggest a large source region, possibly long‐range transport of Asian dust.