A study of near-field radionuclide migration is presented. The study [1] has been performed in the context of the SKB91 study which is a comprehensive performance assessment of disposal of spent fuel. The objective of the present study has been to enable the assessment of which nuclides can be screened out because they decay to insignificant levels already in the near-field of the repository.A numerical model has been used which describes the transient transport of radionuclides through a small hole in a spent fuel canister imbedded in bentonite clay into a fracture in the rock outside the bentonite. Calculations for more than twenty nuclides, nuclides with both high and low solubility, have been made. The effect of sorption in the bentonite backfill is included. Materials data for bentonite where taken from [2]. The size of the penetration hole was assumed to be constant up to the time when the calculations were terminated, 500 000 years after the deposition. The mass transport rate is controlled by diffusion. The model is three dimensional.This paper describes the geometry of the modelled system, the assumptions concerning the transport resistances at the boundary conditions, the handling of the source term and obtained release curves.
Much effort is currently centred on the construction of elaborate computer programs to model the release to the biosphere of radionuclides from proposed high level radioactive waste repositories in deep geological formations. Although the lack or poor quality of background data is often emphasised, it is generally considered that by examining a wide range of possible values of the important parameters involved, likely processes are assessed or their omission and possible relevence is acknowledged. However, one factor that has been almost totally ignored is the presence of micro-organisms in deep geological formations. The common assumption is that the biosphere is limited to the earth's surface, and soil to a depth of a few metres. Recent research has shown, however, that viable micro-organisms can inhabit deep groundwaters and that the biosphere can extend to depths of at least 5 km. Examples of organisms tolerant to extreme environments are given in Table 1 although ranges are likely to be conservative due to the difficulties of culturing these organisms, which tend to have exotic nutritional requirements, and sampling them in extremely hostile environments.
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