The effective desalination and purification devices for seawater/ brackish water treatment are crucial in sustainable progress. Techniques that render high salt removal efficiency and water purification ability at low applied potentials play a central role in sustainable water supplies. One of them is capacitive deionization (CDI) which has drawn significant consideration as a promising deionization technology since the last decade. Desalination efficiency profoundly depends on the utilized electrode material. The most widely used CDI electrodes are carbons due to their cost effectiveness and good stability. However, to acquire high electrosorption capacity, extensive researches are reported with modified carbon materials. CDI cell architectures are equally important for practical high salt removal performance. This review focuses on carbon materials in CDI along with other emerging trends in diverse carbon types, e.g., carbon nanotubes and their composites. Various architectures reported in the literature to improve desalination efficiency are also included here.

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